Spatial variation of PM2.5, PM10, PM2.5 absorbance and PMcoarse concentrations between and within 20 European study areas and the relationship with NO2 - Results of the ESCAPE project

Επιστημονική δημοσίευση - Άρθρο Περιοδικού uoadl:3058119 16 Αναγνώσεις

Μονάδα:
Ερευνητικό υλικό ΕΚΠΑ
Τίτλος:
Spatial variation of PM2.5, PM10, PM2.5 absorbance and PMcoarse concentrations between and within 20 European study areas and the relationship with NO2 - Results of the ESCAPE project
Γλώσσες Τεκμηρίου:
Αγγλικά
Περίληψη:
The ESCAPE study (European Study of Cohorts for Air Pollution Effects) investigates relationships between long-term exposure to outdoor air pollution and health using cohort studies across Europe. This paper analyses the spatial variation of PM2.5, PM2.5 absorbance, PM10 and PMcoarse concentrations between and within 20 study areas across Europe.We measured NO2, NOx, PM2.5, PM2.5 absorbance and PM10 between October 2008 and April 2011 using standardized methods. PMcoarse was determined as the difference between PM10 and PM2.5. In each of the twenty study areas, we selected twenty PM monitoring sites to represent the variability in important air quality predictors, including population density, traffic intensity and altitude. Each site was monitored over three 14-day periods spread over a year, using Harvard impactors. Results for each site were averaged after correcting for temporal variation using data obtained from a reference site, which was operated year-round.Substantial concentration differences were observed between and within study areas. Concentrations for all components were higher in Southern Europe than in Western and Northern Europe, but the pattern differed per component with the highest average PM2.5 concentrations found in Turin and the highest PMcoarse in Heraklion. Street/urban background concentration ratios for PMcoarse (mean ratio 1.42) were as large as for PM2.5 absorbance (mean ratio 1.38) and higher than those for PM2.5 (1.14) and PM10 (1.23), documenting the importance of non-tailpipe emissions. Correlations between components varied between areas, but were generally high between NO2 and PM2.5 absorbance (average R2 = 0.80). Correlations between PM2.5 and PMcoarse were lower (average R2 = 0.39). Despite high correlations, concentration ratios between components varied, e.g. the NO2/PM2.5 ratio varied between 0.67 and 3.06.In conclusion, substantial variability was found in spatial patterns of PM2.5, PM2.5 absorbance, PM10 and PMcoarse. The highly standardized measurement of particle concentrations across Europe will contribute to a consistent assessment of health effects across Europe. © 2012 Elsevier Ltd.
Έτος δημοσίευσης:
2012
Συγγραφείς:
Eeftens, M.
Tsai, M.-Y.
Ampe, C.
Anwander, B.
Beelen, R.
Bellander, T.
Cesaroni, G.
Cirach, M.
Cyrys, J.
de Hoogh, K.
De Nazelle, A.
de Vocht, F.
Declercq, C.
Dedele, A.
Eriksen, K.
Galassi, C.
Gražulevičiene, R.
Grivas, G.
Heinrich, J.
Hoffmann, B.
Iakovides, M.
Ineichen, A.
Katsouyanni, K.
Korek, M.
Krämer, U.
Kuhlbusch, T.
Lanki, T.
Madsen, C.
Meliefste, K.
Mölter, A.
Mosler, G.
Nieuwenhuijsen, M.
Oldenwening, M.
Pennanen, A.
Probst-Hensch, N.
Quass, U.
Raaschou-Nielsen, O.
Ranzi, A.
Stephanou, E.
Sugiri, D.
Udvardy, O.
Vaskövi, É.
Weinmayr, G.
Brunekreef, B.
Hoek, G.
Περιοδικό:
ATMOSPHERIC ENVIRONMENT
Τόμος:
62
Σελίδες:
303-317
Λέξεις-κλειδιά:
Coarse particles; PM2.5; Soot; Spatial variations; Traffic, absorption; altitude; atmospheric pollution; background level; concentration (composition); health impact; health risk; nitrogen oxides; particle size; particulate matter; pollution exposure; population density; soot; spatial variation; temporal variation; traffic emission, air quality; altitude; article; concentration (parameters); Europe; particulate matter; population density; priority journal; traffic, Europe
Επίσημο URL (Εκδότης):
DOI:
10.1016/j.atmosenv.2012.08.038
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